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Accelerated Microbial Reduction of Azo Dye by Using Biochar from Iron-Rich-Biomass Pyrolysis | |
Tan, Wenbing1; Wang, Lei1; Yu, Hanxia2; Zhang, Hui1; Zhang, Xiaohui1; Jia, Yufu3; Li, Tongtong4; Dang, Qiuling1; Cui, Dongyu1; Xi, Beidou1 | |
2019 | |
发表期刊 | MATERIALS |
ISSN | 1996-1944 |
卷号 | 12期号:7 |
摘要 | Biochar is widely used in the environmental-protection field. This study presents the first investigation of the mechanism of biochar prepared using iron (Fe)-rich biomass and its impact on the reductive removals of Orange G dye by Shewanella oneidensis MR-1. The results show that biochars significantly accelerated electron transfer from cells to Orange G and thus stimulated reductive removal rate to 72-97%. Both the conductive domains and the charging and discharging of surface functional groups in biochars played crucial roles in the microbial reduction of Orange G to aniline. A high Fe content of the precursor significantly enhanced the conductor performance of the produced biochar and thus enabled the biochar to have a higher reductive removal rate of Orange G (97%) compared to the biochar prepared using low-Fe precursor (75%), but did not promote the charging and discharging capacity of the produced biochar. This study can prompt the search for natural biomass with high Fe content to confer the produced biochar with wide-ranging applications in stimulating the microbial reduction of redox-active pollutants. |
关键词 | Orange G dye biochar iron-rich-stalk pyrolysis microbial reduction electron transfer |
学科领域 | Chemistry, Physical ; Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering ; Physics, Applied ; Physics, Condensed Matter |
DOI | 10.3390/ma12071079 |
收录类别 | SCI |
语种 | 英语 |
WOS关键词 | PHOTOCATALYTIC DEGRADATION ; ELECTRICITY PRODUCTION ; ELECTRON-TRANSFER ; FENTON PROCESSES ; AQUEOUS-SOLUTION ; LOW-COST ; CARBON ; REMOVAL ; DECOLORIZATION ; WATER |
WOS研究方向 | Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering ; Physics |
WOS记录号 | WOS:000465500700078 |
出版者 | MDPI |
文献子类 | Article |
出版地 | BASEL |
资助机构 | National Key Research and Development Program of China [2018YFC1900102] ; Major Science and Technology Program for Water Pollution Control and Treatment [2012ZX07203-003] ; Beijing Advanced Innovation Center for Future Urban Design of Beijing University of Civil Engineering and Architecture [UDC 2017032512] |
作者邮箱 | wenbingtan@126.com ; wangleicraes@163.com ; yhanxia@126.com ; zhanghuiguom@163.com ; baixue215@163.com ; yufu123jia@163.com ; 18811785922@163.com ; dangling819@126.com ; cuidy@craes.org.cn ; wbtann@126.com |
作品OA属性 | Green Published, gold, Green Submitted |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ibcas.ac.cn/handle/2S10CLM1/19804 |
专题 | 植被与环境变化国家重点实验室 |
作者单位 | 1.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China 2.Chinese Res Inst Environm Sci, State Environm Protect Key Lab Simulat & Control, Beijing 100012, Peoples R China 3.South China Normal Univ, Sch Life Sci, Guangzhou 510631, Guangdong, Peoples R China 4.Chinese Acad Sci, Inst Bot, State Key Lab Vegetat & Environm Change, Beijing 100093, Peoples R China 5.Capital Normal Univ, Coll Resource Environm & Tourism, Beijing 100048, Peoples R China |
推荐引用方式 GB/T 7714 | Tan, Wenbing,Wang, Lei,Yu, Hanxia,et al. Accelerated Microbial Reduction of Azo Dye by Using Biochar from Iron-Rich-Biomass Pyrolysis[J]. MATERIALS,2019,12(7). |
APA | Tan, Wenbing.,Wang, Lei.,Yu, Hanxia.,Zhang, Hui.,Zhang, Xiaohui.,...&Xi, Beidou.(2019).Accelerated Microbial Reduction of Azo Dye by Using Biochar from Iron-Rich-Biomass Pyrolysis.MATERIALS,12(7). |
MLA | Tan, Wenbing,et al."Accelerated Microbial Reduction of Azo Dye by Using Biochar from Iron-Rich-Biomass Pyrolysis".MATERIALS 12.7(2019). |
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Tan-2019-Accelerated(2052KB) | 期刊论文 | 出版稿 | 开放获取 | CC BY-NC-SA | 浏览 请求全文 |
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