Photoelectrochemical Complexes of Fucoxanthin-Chlorophyll Protein for Bio-Photovoltaic Conversion with a High Open-Circuit Photovoltage

doi:10.1016/j.ympev.2016.12.026

IB-CAS > 中科院光生物学重点实验室

	Photoelectrochemical Complexes of Fucoxanthin-Chlorophyll Protein for Bio-Photovoltaic Conversion with a High Open-Circuit Photovoltage
	Zhang, Tianning 3; Liu, Cheng 1; Dong, Wenjing 2; Wang, Wenda 1; Sun, Yan ; Chen, Xin 3; Yang, Chunhong 1; Dai, Ning 3,4
	2017
发表期刊	CHEMISTRY-AN ASIAN JOURNAL
ISSN	1861-4728
卷号	12 期号:23 页码:2996-2999
摘要	Open-circuit photovoltage (V-oc) is among the critical parameters for achieving an efficient light-to-charge conversion in existing solar photovoltaic devices. Natural photosynthesis exploits light-harvesting chlorophyll (Chl) protein complexes to transfer sunlight energy efficiently. We describe the exploitation of photosynthetic fucoxanthin-chlorophyll protein (FCP) complexes for realizing photoelectrochemical cells with a high V-oc. An antenna-dependent photocurrent response and a V-oc up to 0.72V are observed and demonstrated in the bio-photovoltaic devices fabricated with photosynthetic FCP complexes and TiO2 nanostructures. Such high V-oc is determined by fucoxanthin in FCP complexes, and is rarely found in photoelectrochemical cells with other natural light-harvesting antenna. We think that the FCP-based bio-photovoltaic conversion will provide an opportunity to fabricate environmental benign photoelectrochemical cells with high V-oc, and also help improve the understanding of the essential physics behind the light-to-charge conversion in photosynthetic complexes.
关键词	fucoxanthin-chlorophyll protein light-to-charge conversion photoelectrochemical cells photosynthesis photovoltage
学科领域	Biochemistry & Molecular Biology ; Evolutionary Biology ; Genetics & Heredity
DOI	10.1016/j.ympev.2016.12.026
收录类别	SCI
语种	英语
WOS关键词	SENSITIZED SOLAR-CELLS ; EXCITATION-ENERGY-TRANSFER ; LIGHT-HARVESTING COMPLEX ; NANOROD ARRAYS ; EXCITED-STATES ; ELECTRONIC COHERENCE ; WATER OXIDATION ; DYNAMICS ; TIO2 ; BIOPHOTOVOLTAICS
WOS记录号	WOS:000394200500054
出版者	WILEY-V C H VERLAG GMBH
文献子类	Article
出版地	WEINHEIM
EISSN	1861-471X
资助机构	National Key R&D Program of China [2016YFA0202201, 2017YFA0503701] ; Strategic Priority Research Program of the Chinese Academy of SciencesChinese Academy of Sciences [XDB17030100] ; NSFCNational Natural Science Foundation of China (NSFC) [61376016, 61290304, 31570236, 31370275] ; CASChinese Academy of Sciences [KSZD-EW-Z-018] ; Youth Innovation Promotion Association CAS
作者邮箱	ndai@mail.sitp.ac.cn ; yangch@ibcas.ac.cn ; xinchen@mail.sitp.ac.cn
引用统计	被引频次：16[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.ibcas.ac.cn/handle/2S10CLM1/22115
专题	中科院光生物学重点实验室
作者单位	1.Chinese Acad Sci, Natl Lab Infrared Phys, Shanghai Inst Tech Phys, Shanghai 200083, Peoples R China 2.Chinese Acad Sci, Key Lab Photobiol, Inst Bot, Beijing 100093, Peoples R China 3.Hubei Univ, Hubei Collaborat Innovat Ctr Adv Organ Chem Mat, Fac Phys & Elect Sci, Wuhan 430062, Hubei, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 5.Jiangsu Collaborat Innovat Ctr Photovolta Sci & E, Changzhou 213164, Peoples R China
推荐引用方式 GB/T 7714	Zhang, Tianning,Liu, Cheng,Dong, Wenjing,et al. Photoelectrochemical Complexes of Fucoxanthin-Chlorophyll Protein for Bio-Photovoltaic Conversion with a High Open-Circuit Photovoltage[J]. CHEMISTRY-AN ASIAN JOURNAL,2017,12(23):2996-2999.
APA	Zhang, Tianning.,Liu, Cheng.,Dong, Wenjing.,Wang, Wenda.,Sun, Yan.,...&Dai, Ning.(2017).Photoelectrochemical Complexes of Fucoxanthin-Chlorophyll Protein for Bio-Photovoltaic Conversion with a High Open-Circuit Photovoltage.CHEMISTRY-AN ASIAN JOURNAL,12(23),2996-2999.
MLA	Zhang, Tianning,et al."Photoelectrochemical Complexes of Fucoxanthin-Chlorophyll Protein for Bio-Photovoltaic Conversion with a High Open-Circuit Photovoltage".CHEMISTRY-AN ASIAN JOURNAL 12.23(2017):2996-2999.

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