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Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid
Wang, Wangyin; Wang, Hong1; Zhu, Qingjun1; Qin, Wei; Han, Guangye; Shen, Jian-Ren; Zong, Xu; Li, Can
2016
发表期刊ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
ISSN1433-7851
卷号55期号:32页码:9229-9233
摘要Integrating natural and artificial photosynthetic platforms is an important approach to developing solar-driven hybrid systems with exceptional function over the individual components. A natural-artificial photosynthetic hybrid platform is formed by wiring photosystem II (PSII) and a platinum-decorated silicon photoelectrochemical (PEC) cell in a tandem manner based on a photocatalytic-PEC Z-scheme design. Although the individual components cannot achieve overall water splitting, the hybrid platform demonstrated the capability of unassisted solar-driven overall water splitting. Moreover, H-2 and O-2 evolution can be separated in this system, which is ascribed to the functionality afforded by the unconventional Z-scheme design. Furthermore, the tandem configuration and the spatial separation between PSII and artificial components provide more opportunities to develop efficient natural-artificial hybrid photosynthesis systems.
关键词photocatalysis photoelectrochemistry photosystem II water splitting Z-scheme
学科领域Chemistry, Multidisciplinary
DOI10.1002/anie.201604091
收录类别SCI
语种英语
WOS关键词PHOTO-BIOELECTROCHEMICAL CELLS ; SHUTTLE REDOX MEDIATOR ; VISIBLE-LIGHT ; ELECTRON-TRANSFER ; Z-SCHEME ; OXYGEN ; SOLAR ; PHOTOCATALYSTS ; SYSTEM ; RESOLUTION
WOS研究方向Science Citation Index Expanded (SCI-EXPANDED)
WOS记录号WOS:000383371800017
出版者WILEY-V C H VERLAG GMBH
文献子类Article
出版地WEINHEIM
EISSN1521-3773
资助机构973 National Basic Research Program of the Ministry of Science and TechnologyNational Basic Research Program of China [2014CB239403] ; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21090340] ; Key Research Program of the Chinese Academy of Science [KGZD-EW-T05] ; Young Thousand Talents Program of China
作者邮箱xzong@dicp.ac.cn ; canli@dicp.ac.cn
引用统计
被引频次:49[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ibcas.ac.cn/handle/2S10CLM1/25304
专题中科院光生物学重点实验室
作者单位1.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat IChEM, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,Dalian Inst Chem Phys, Zhongshan Rd 457, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Inst Bot, Key Lab Photobiol, Photosynthesis Res Ctr, Beijing 100093, Peoples R China
4.Okayama Univ, Grad Sch Nat Sci & Technol, Photosynthesis Res Ctr, 1-1 Naka 3 Chome, Okayama 7008530, Japan
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GB/T 7714
Wang, Wangyin,Wang, Hong,Zhu, Qingjun,et al. Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(32):9229-9233.
APA Wang, Wangyin.,Wang, Hong.,Zhu, Qingjun.,Qin, Wei.,Han, Guangye.,...&Li, Can.(2016).Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(32),9229-9233.
MLA Wang, Wangyin,et al."Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.32(2016):9229-9233.
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