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Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid | |
Wang, Wangyin; Wang, Hong1; Zhu, Qingjun1; Qin, Wei; Han, Guangye; Shen, Jian-Ren; Zong, Xu; Li, Can | |
2016 | |
发表期刊 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION |
ISSN | 1433-7851 |
卷号 | 55期号:32页码:9229-9233 |
摘要 | Integrating natural and artificial photosynthetic platforms is an important approach to developing solar-driven hybrid systems with exceptional function over the individual components. A natural-artificial photosynthetic hybrid platform is formed by wiring photosystem II (PSII) and a platinum-decorated silicon photoelectrochemical (PEC) cell in a tandem manner based on a photocatalytic-PEC Z-scheme design. Although the individual components cannot achieve overall water splitting, the hybrid platform demonstrated the capability of unassisted solar-driven overall water splitting. Moreover, H-2 and O-2 evolution can be separated in this system, which is ascribed to the functionality afforded by the unconventional Z-scheme design. Furthermore, the tandem configuration and the spatial separation between PSII and artificial components provide more opportunities to develop efficient natural-artificial hybrid photosynthesis systems. |
关键词 | photocatalysis photoelectrochemistry photosystem II water splitting Z-scheme |
学科领域 | Chemistry, Multidisciplinary |
DOI | 10.1002/anie.201604091 |
收录类别 | SCI |
语种 | 英语 |
WOS关键词 | PHOTO-BIOELECTROCHEMICAL CELLS ; SHUTTLE REDOX MEDIATOR ; VISIBLE-LIGHT ; ELECTRON-TRANSFER ; Z-SCHEME ; OXYGEN ; SOLAR ; PHOTOCATALYSTS ; SYSTEM ; RESOLUTION |
WOS研究方向 | Science Citation Index Expanded (SCI-EXPANDED) |
WOS记录号 | WOS:000383371800017 |
出版者 | WILEY-V C H VERLAG GMBH |
文献子类 | Article |
出版地 | WEINHEIM |
EISSN | 1521-3773 |
资助机构 | 973 National Basic Research Program of the Ministry of Science and TechnologyNational Basic Research Program of China [2014CB239403] ; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21090340] ; Key Research Program of the Chinese Academy of Science [KGZD-EW-T05] ; Young Thousand Talents Program of China |
作者邮箱 | xzong@dicp.ac.cn ; canli@dicp.ac.cn |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ibcas.ac.cn/handle/2S10CLM1/25304 |
专题 | 中科院光生物学重点实验室 |
作者单位 | 1.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat IChEM, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,Dalian Inst Chem Phys, Zhongshan Rd 457, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst Bot, Key Lab Photobiol, Photosynthesis Res Ctr, Beijing 100093, Peoples R China 4.Okayama Univ, Grad Sch Nat Sci & Technol, Photosynthesis Res Ctr, 1-1 Naka 3 Chome, Okayama 7008530, Japan |
推荐引用方式 GB/T 7714 | Wang, Wangyin,Wang, Hong,Zhu, Qingjun,et al. Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(32):9229-9233. |
APA | Wang, Wangyin.,Wang, Hong.,Zhu, Qingjun.,Qin, Wei.,Han, Guangye.,...&Li, Can.(2016).Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(32),9229-9233. |
MLA | Wang, Wangyin,et al."Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.32(2016):9229-9233. |
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